Soutenance de thèse
Yijie Shi
CEREA
Molecular modeling of β-caryophyllene secondary organic aerosols and markers: mechanism development and reduction
Résumé
This thesis studies how β-caryophyllene, a volatile organic compound emitted from natural sources, changes in the atmosphere. When it reacts with oxidants in the air, it undergoes a series of chemical and physical processes that can lead to the formation of secondary organic aerosol (SOA), tiny particles that affect air quality, climate, and human health.
This work develops a new chemical mechanism to better describe how these particles form, grow, and change in composition. The mechanism was tested against published laboratory data and was shown to perform well under different temperatures. The study also identifies the key factors controlling particle formation. The new mechanism was then applied under near-realistic atmospheric conditions to evaluate the potential formation of SOA. Finally, a simplified version of the mechanism was created so that it can be more easily used in large-scale air quality and climate models.
Informations supplémentaires
Location
INERIS, Salle CAMPANULE, Parc Technologique Alata BP 2, 60550 Verneuil-en-Halatte
Online meeting link
Microsoft Teams meeting
Join here: https://teams.microsoft.com/meet/36183110105234?p=18nit697B41hajDyWO
Meeting ID: 361 831 101 052 34
Passcode: oV7xt9pt
Composition du jury
Solène Turquety, Professor, LATMOS, Sorbonne University
Alexandre Tomas, Professor, CERI EE, IMT Nord Europe
Barbara D’Anna, Research Director, LCE, Aix-Marseille University
Laurent Deguillaume, Physicist, OPGC, Clermont Auvergne University
Didier Hauglustaine, Research Director, LSCE, Paris-Saclay University
Karine Sartelet, Professor, CEREA, ENPC, IPParis
Florian Couvidat, INERIS